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Temperature dependence of Peierls–Hubbard phase transition in [Pd(cptn)2Br]Br2 studied by scanning tunneling microscopy
http://hdl.handle.net/2241/00143754
77901fdc-c5c2-49fd-b24e-e1b38337450d
名前 / ファイル | ライセンス | Actions | |
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item type | Journal Article(1) | |||||
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公開日 | 2016-09-01 | |||||
タイトル | ||||||
タイトル | Temperature dependence of Peierls–Hubbard phase transition in [Pd(cptn)2Br]Br2 studied by scanning tunneling microscopy | |||||
言語 | ||||||
言語 | eng | |||||
資源タイプ | ||||||
タイプ | journal article | |||||
著者 |
Hosomi, Yuka
× Hosomi, Yuka× Yoshida, Shoji× Taninaka, Atsushi× Yoshida, Takefumi× Takaishi, Shinya× Takeuchi, Osamu× Yamashita, Masahiro× Shigekawa, Hidemi |
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著者別名 |
吉田, 昭二
× 吉田, 昭二× 谷中, 淳× 武内, 修× 重川, 秀実 |
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抄録 | ||||||
内容記述 | The temperature dependence of the Peierls–Hubbard phase transition in [Pd(cptn)2Br]Br2 (cptn: 1R,2R-diaminocyclopentane) was directly observed using a low-temperature scanning tunneling microscope. A short ligand without alkyl chains was used to form a rigid crystal lattice to reduce the effect of structural changes in the crystal with temperature. The hysteresis in the temperature dependence of the ratio between the areas of the charge density wave (CDW) state produced by the PdII–PdIV mixed-valence state and the Mott–Hubbard (MH) state with a PdIII-averaged valence state which is a characteristic of the first-order phase transition, was directly observed at the atomic scale. Pinning of the CDW phase by defects was observed below the critical temperature, suggesting the growth of the CDW phase with defects as nuclei. | |||||
書誌情報 |
Japanese journal of applied physics 巻 55, 号 8S1, p. 08NB16, 発行日 2016-08 |
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ISSN | ||||||
収録物識別子 | 0021-4922 | |||||
書誌レコードID | ||||||
収録物識別子 | AA12295836 | |||||
DOI | ||||||
関連識別子 | ||||||
関連識別子 | 10.7567/JJAP.55.08NB16 | |||||
権利 | ||||||
権利情報 | © 2016 The Japan Society of Applied Physics | |||||
著者版フラグ | ||||||
値 | author | |||||
出版者 | ||||||
出版者 | The Japan Society of Applied Physics |