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Mechanically activated switching of Si-based single-molecule junction as imaged with three-dimensional dynamic probe
http://hdl.handle.net/2241/00132408
d4c1dcf2-cae2-46a5-aaae-4f106711d8d1
名前 / ファイル | ライセンス | Actions | |
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item type | Journal Article(1) | |||||
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公開日 | 2016-01-06 | |||||
タイトル | ||||||
タイトル | Mechanically activated switching of Si-based single-molecule junction as imaged with three-dimensional dynamic probe | |||||
言語 | ||||||
言語 | eng | |||||
資源タイプ | ||||||
タイプ | journal article | |||||
著者 |
Nakamura, Miki
× Nakamura, Miki× Yoshida, Shoji× Katayama, Tomoki× Taninaka, Atsushi× Mera, Yutaka× Okada, Susumu× Takeuchi, Osamu× Shigekawa, Hidemi |
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著者別名 |
吉田, 昭二
× 吉田, 昭二× 谷中, 淳× 岡田, 晋× 武内, 修× 重川, 秀実 |
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抄録 | ||||||
内容記述 | Understanding and extracting the full functions of single-molecule characteristics are key factors in the development of future device technologies, as well as in basic research on molecular electronics. Here we report a new methodology for realizing a three-dimensional (3D) dynamic probe of single-molecule conductance, which enables the elaborate 3D analysis of the conformational effect on molecular electronics, by the formation of a Si/single molecule/Si structure using scanning tunnelling microscopy (STM). The formation of robust covalent bonds between a molecule and Si electrodes, together with STM-related techniques, enables the stable and repeated control of the conformational modulation of the molecule. By 3D imaging of the conformational effect on a 1,4-diethynylbenzene molecule, a binary change in conductance with hysteresis is observed for the first time, which is considered to originate from a mechanically activated conformational change. | |||||
書誌情報 |
Nature Communications 巻 6, p. 8465, 発行日 2015-10 |
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ISSN | ||||||
収録物識別子 | 2041-1723 | |||||
書誌レコードID | ||||||
収録物識別子 | AA12645905 | |||||
PubMed番号 | ||||||
関連識別子 | ||||||
関連識別子 | 26439280 | |||||
DOI | ||||||
関連識別子 | ||||||
関連識別子 | 10.1038/ncomms9465 | |||||
権利 | ||||||
権利情報 | © 2015 Macmillan Publishers Limited. All rights reserved. This work is licensed under a Creative Commons Attribution 4.0 International License. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in the credit line; if the material is not included under the Creative Commons license, users will need to obtain permission from the license holder to reproduce the material. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ | |||||
著者版フラグ | ||||||
値 | publisher | |||||
出版者 | ||||||
出版者 | Nature Publishing Group |