@article{oai:tsukuba.repo.nii.ac.jp:00028088, author = {長谷, 宗明 and Hase, Muneaki and Katsuragawa, Masayuki and Constantinescu, Anca Monia and Petek, Hrvoje}, issue = {4}, journal = {Nature photonics}, month = {Apr}, note = {High-order nonlinear light–matter interactions in gases enable the generation of X-ray and attosecond light pulses, metrology and spectroscopy1. Optical nonlinearities in solid-state materials are particularly interesting for combining optical and electronic functions for high-bandwidth information processing2. Third-order nonlinear optical processes in silicon have been used to process optical signals with bandwidths greater than 1 GHz (ref. 2). However, fundamental physical processes for a silicon-based optical modulator in the terahertz bandwidth range have not yet been explored. Here, we demonstrate ultrafast phononic modulation of the optical index of silicon by irradiation with intense few-cycle femtosecond pulses. The anisotropic reflectivity modulation by the resonant Raman susceptibility at the fundamental frequency of the longitudinal optical phonon of silicon (15.6 THz) generates a frequency comb up to seventh order. All-optical >100 THz frequency comb generation is realized by harnessing the coherent atomic motion of the silicon crystalline lattice at its highest mechanical frequency.}, pages = {243--247}, title = {Frequency comb generation at terahertz frequencies by coherent phonon excitation in silicon}, volume = {6}, year = {2012} }